You can do this as long as you can identify different types of access.
For example you can have ppp authentication use RADIUS and telnet authentication use TACACS, or you can have one interface (eg dialer) use RADIUS and another (eg vty) use TACACS between the same router and server.
To achieve this with Cisco Secure NT/2000 you will need to use the ip radius-server/tacacs-server source-interface command to make one router look like two to the server. For Cisco Secure Unix this is not a problem.